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1 article(s) from Hanefeld, Marc

Electron interactions with the heteronuclear carbonyl precursor H₂FeRu₃(CO)₁₃ and comparison with HFeCo₃(CO)₁₂: from fundamental gas phase and surface science studies to focused electron beam induced deposition

Ragesh Kumar T P,
Paul Weirich,
Lukas Hrachowina,
Marc Hanefeld,
Ragnar Bjornsson,
Helgi Rafn Hrodmarsson,
Sven Barth,
D. Howard Fairbrother,
Michael Huth and
Oddur Ingólfsson

Beilstein J. Nanotechnol. 2018, 9, 555–579, doi:10.3762/bjnano.9.53

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Figure 1: Structural arrangement of HFeCo₃(CO)₁₂ and H₂FeRu₃(CO)₁₃ illustrating differences in symmetry and l...

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Figure 2: Isotope distribution of a) HFeCo₃(CO)₁₂ and b) H₂FeRu₃(CO)₁₃. Isotope distribution for both compoun...

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Figure 3: Negative ion yield curves for the formation of a) [Fe(CO)_n]⁻ and b) [Ru(CO)_n]⁻ up on electron attac...

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Figure 4: Loss of Fe(CO)₂ (panel a), Fe(CO)₃ (panel b), Fe(CO)₄ (panel c) and additional loss of up to 7 COs ...

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Figure 5: Negative ions formed through loss of Ru(CO)₃ (panel a), Ru(CO)₄ (panel b) and further loss of up to...

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Figure 6: Calculated spin density of the [H₂FeRu₃(CO)₁₃]⁻ anion; a) in the constrained geometry of neutral H₂...

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Figure 7: Calculated MO diagrams of H₂FeRu₃(CO)₁₃ and HFeCo₃(CO)₁₂. Red lines represent the unoccupied molecu...

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Figure 8: Electron impact ionization spectra of H₂FeRu₃(CO)₁₃ recorded at electron energy of 70 eV, upper pan...

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Figure 9: Evolution of O 1s, Fe 2p and Ru 3d/C 1s XPS regions of a H₂FeRu₃(CO)₁₃ film exposed to electron dos...

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Figure 10: Change in fractional coverage of oxygen atoms (red stars) and, Ru 3d_5/2 peak position (blue open ci...

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Figure 11: Mass spectrum of neutral gas phase species desorbed from an H₂FeRu₃(CO)₁₃ film during the course of...

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Figure 12: Changes in O 1s, Fe 2p and Ru 3d/C 1s XPS regions when an H₂FeRu₃(CO)₁₃ film was exposed to electro...

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Figure 13: Initial decomposition/deposition of surface adsorbed H₂FeRu₃(CO)₁₃ precursor, mediated by dissociat...

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Figure 14: Schematic showing the incorporation of partially decarbonylated intermediate of H₂FeRu₃(CO)₁₃ into ...

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Figure 15: (a) AFM cross sections of deposits shown in the SEM micrograph (b) at the positions indicated by th...

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Figure 16: Transport measurements of as-grown Fe–Ru deposit and deposits grown under identical conditions afte...

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Published 14 Feb 2018

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Electron interactions with the heteronuclear carbonyl precursor H2FeRu3(CO)13 and comparison with HFeCo3(CO)12: from fundamental gas phase and surface science studies to focused electron beam induced deposition

Electron interactions with the heteronuclear carbonyl precursor H₂FeRu₃(CO)₁₃ and comparison with HFeCo₃(CO)₁₂: from fundamental gas phase and surface science studies to focused electron beam induced deposition